R. Lu et al., RESONANT QUANTUM COHERENCE OF THE NEEL VECTOR IN A MAGNETIC-FIELD APPLIED ALONG THE MEDIUM AXIS, Physical review. B, Condensed matter, 58(13), 1998, pp. 8542-8548
Based on the two-sublattice model. we study the topological phase inte
rference effect in resonant macroscopic quantum coherence of the Neel
vector in a single-domain antiferromagnetic nanoparticle with biaxial
crystal symmetry placed in an external magnetic field a;;plied along t
he medium axis. By applying the standard instanton technique in spin-c
oherent-state path integral, we evaluate both the Wentzel-Kramers-Bril
louin exponent and the preexponential factors in the instanton's contr
ibution to the tunneling-level splitting. The Euclidean transition amp
litude is obtained by making use of the dilute instanton-gas approxima
tion. The low-lying tunneling-level spectrum and the thermodynamic pro
perties of magnetic tunneling states are found to depend on the parity
of the excess spin of the antiferromagnetic nanoparticle significantl
y. possible relevance to experiments is also discussed.