S. Itoh et al., SPIN DYNAMICS IN 2-DIMENSIONAL PERCOLATING HEISENBERG ANTIFERROMAGNETS, Journal of the Physical Society of Japan, 67(10), 1998, pp. 3610-3616
Inelastic neutron-scattering experiments were performed on two-dimensi
onal Heisenberg antiferromagnets, Rb2MncMg1-cF4, with the magnetic con
centrations (c = 0.598 and 0.516) just above and below the percolation
threshold (c(p) = 0.593 for the square lattice). Also, the magnetic r
esponse (chi '' (q, E)) was investigated over a wide temperature range
. We observed an overdamped chi '' (q, E), which was well fitted to a
damped harmonic-oscillator scattering function. At low temperatures, c
hi '' (q, E) is dispersive and can be described by the predicted funct
ional form of fracton excitations. As the temperature increases, the q
-dependence gradually becomes weaker, and chi '' (q, E) almost becomes
independent of q at temperatures higher than 150 K. The incoherent ch
aracter of chi '' (q, E) at high temperatures indicates that collectiv
e motions do not exist due to very small thermal correlation lengths.
Fracton excitations exist only at low temperatures.