M. Salvatores et al., THE TRANSMUTATION OF LONG-LIVED FISSION-PRODUCTS BY NEUTRON-IRRADIATION, Nuclear science and engineering, 130(3), 1998, pp. 309-319
A general physical approach and simplified algorithm have been develop
ed that allow utilities to choose their strategy for treatment of the
most dangerous long-lived fission products (either to incinerate under
neutron flux or to store in underground repository) as well as to ass
ess the overall neutron consumption needed for their incineration in a
fast neutron spectrum, it has been demonstrated that if nuclear power
can solve transuranic (TRU) waste transmutation problems and be able
to incinerate the mast toxic long-lived nuclides, such as Tc, I, and C
s (it demands -0.15 n/fission for all these nuclides without isotopic
separation), then the long-term radiotoxicity in the underground repos
itory will not exceed the initial radiotoxicity of uranium fuel. This
is one of the most important criteria of the radiologically clean nucl
ear power concept. Hence, apart from TRU transmutation problems, the e
mphasis is now on long-lived fission product incineration.