We present the windowed Fourier transform or vibrogram of 960 experime
ntal vibrational levels of CS2 up to 19150 cm(-1). The averaged vibrog
ram shows the evolution of the correlation hole. Then the dynamics at
short times is investigated by the periodic orbit theory. The first re
currences of the vibrogram are assigned in terms of winding numbers of
an integrable 3D resonance model.