We simulate the behaviour of suspensions of large-particle, non-Browni
an, neutrally-buoyant spheres in a Newtonian liquid with a Galerkin, f
inite element, Navier-Stokes solver into which is incorporated a conti
nuum constitutive relationship described by Phillips et al. (1992). Th
is constitutive description couples a Newtonian stress/shear-rate rela
tionship (where the local viscosity of the suspension is dependent on
the local volume fraction of solids) with a shear-induced migration mo
del of the suspended particles. The two-dimensional and three-dimensio
nal (axisymmetric) model is benchmarked with a variety of single-phase
and two-phase analytic solutions and experimental results. We describ
e new experimental results using nuclear magnetic resonance imaging to
determine non-invasively the evolution of the solids-concentration pr
ofiles of initially well-mixed suspensions as they separate when subje
cted to slow flow between counter-rotating eccentric cylinders and to
piston-driven flow in a pipe. We show good qualitative and quantitativ
e agreement of the numerical predictions and the experimental measurem
ents. These flows result in complex final distributions of the solids,
causing rheological behaviour that cannot be accurately described wit
h typical single-phase constitutive equations.