ON AMPLIFICATION OF RADIATION EMITTED FROM THE EXCITED AUTOIONIZING STATE OF THE H-2 MOLECULE IN THE PRESENCE OF INCOHERENT PUMPING TO THE LOWEST AUTOIONIZING STATE
L. Adhya et al., ON AMPLIFICATION OF RADIATION EMITTED FROM THE EXCITED AUTOIONIZING STATE OF THE H-2 MOLECULE IN THE PRESENCE OF INCOHERENT PUMPING TO THE LOWEST AUTOIONIZING STATE, Nuovo cimento della Societa italiana di fisica. D, Condensed matter,atomic, molecular and chemical physics, biophysics, 20(9), 1998, pp. 1283-1294
We have shown that the amplification without population inversion (AWO
PI) from the fu st excited autoionizing (AI) state of the (1)Sigma(g)
symmetry of the H-2 molecules can be obtained when the lowest AI state
of the (1)Sigma(g) symmetry is pumped incoherently. We have considere
d a resonant two-photon transition scheme from the ground X(1)Sigma(g)
(v = 0; j = 1) state to the ionization continuum embracing the two AI
states (the lowest and the first excited autoionizing states) of the
(1)Sigma(g) symmetry via the resonant intermediate B(1)Sigma(u) (v = 4
, j = 2) level. The effect of two-photon near-resonant autoionizing ch
annels via the near-resonant rovibrational levels of the B(1)Sigma(u)
state has also been considered. We have found that the gain can be obt
ained in different spectral regions corresponding to the resonances wi
th the lowest and first excited AI states from the inter mediate level
s of the B(1)Sigma(u) state. The inherent coherence between two AI sta
tes due to the configuration interaction coupling via the common conti
nuum has been found to have a significant effect on the amplification
process, which occurs around all the resonance frequencies connecting
this AI state with the intermediate levels. This gain can be significa
ntly modified by increasing the coupling strength of this excited AI s
tate with the continuum, Moreover, the gain from the excited AI state
remains unaffected by the damping caused by incoherent pumping to the
lowest AI state. It has also been shown that the persistence of invers
ionless gain from the excited AI state is shorter than that from the l
owest Al state. The presence of close-lying near-resonant rovibrationa
l levels leads to the increase in gain around the resonances with two
AI states from the B(1)Sigma(u) (v = 4, j = 2) level. The advantages o
f this type of scheme are: i) AWOPI can be obtained from an excited AI
state although it has not been pumped and ii) the amplification obtai
ned from the excited AI state is almost unaffected by the distortion c
aused by incoherent pumping to the lower AI state.