Bk. Roul, Gamma ray irradiation effects on electrical transport and microwave properties of BISCO superconducting films, J SUPERCOND, 12(2), 1999, pp. 409-416
High-T-c Superconducting films of Bi-Sr-Ca-Cu-O (2:2:1:2) have been synthes
ized by spray pyrolysis of nitrate precursors onto yttria stabilized zircon
ia (YSZ). gamma-ray irradiation of the sample, was carried out using a Co-6
0 source Of 10(3) Ci Strength for several hundreds of hours; the dose recei
ved by the samples was 80 K rad/hr. Superconducting properties such as crit
ical transition temperature (T-c), resistivity (KR), critical current densi
ty (J(tc)). Voltage-time relaxation (Vt) and microwave induced de voltage w
ere investigated as a function of temperature down to 77 K after gamma-ray
irradiation. gamma-ray irradiation was found to have practically no effect
on its structural modification and on the critical transition temperature.
However, transport critical current density (J(tc)) increased. The increase
of pinning energies with irradiation suggests that these changes in proper
ties are dominated by radiation-induced randomly distributed mobile oxygen
defects in the films. An appreciable decrease in the microwave-induced dc v
oltage at 77 K was also observed after irradiation which suggests that the
mobile defects are clustered at the major defect region and reduce the tota
l number of weak links. These results suggests that oxygen defects induced
by gamma-ray irradiation of BISCO films act as important and major pinning
centers which is responsible for the enhancement of J(tc) and reduction of
microwave induced dc voltage.