We report on the growth of epitaxial La2/3Sr1/3MnO3 thin films on buffered
Si(001) substrates. We show that a suitable choice of the buffer heterostru
cture allows one to obtain epitaxial (00h), (0hh), and (hhh) manganite thin
films. The magnetotransport properties are investigated and we have found
that the low-field magnetoresistance is directly related to the width of th
e normal-to-plane rocking curves, irrespective of the film orientation. The
magnetic anisotropy of these films has also been determined. (C) 1999 Amer
ican Institute of Physics. [S0021-8979(99)35108-2].