Molecular beam epitaxy has been used to stabilize FexCo1-x alloy films over
the entire composition range on diamond (100) substrates. Below a critical
thickness, the films are single crystal face-centered-cubic (fcc) as deter
mined from reflection high energy electron diffraction. Superconducting qua
ntum interference device magnetometry studies reveal a nonmonotonic increas
e in the magnetization of the fcc alloys with Fe concentration, while ferro
magnetic resonance indicates a small magnetic anisotropy for x>20%. (C) 199
9 American Institute of Physics. [S0021-8979(99)64808-3].