We present a compilation of data for all 258 gamma-ray flares detected abov
e 300 keV by the Gamma Ray Spectrometer (GRS) aboard the Solar Maximum Miss
ion satellite. This gamma-ray flare sample was collected during the period
from 1980 February to 1989 November; covering the latter half of the 21st s
olar sunspot cycle and the onset of the 22d solar sunspot cycle. We describ
e the SMM/GRS instrument, its in-orbit operation, and the principal data re
duction methods used to derive the gamma-ray flare properties. Utilizing me
asurements for 185 flares that were sufficiently intense to allow the deriv
ation of gamma-ray spectra, we present an atlas of time profiles and gamma-
ray spectra. The flare parameters derived from the gamma-ray spectra includ
e bremsstrahlung fluence and best-fit power-law parameters, narrow nuclear
line fluence, positron annihilation line fluence, neutron capture line flue
nce, and an indication of whether or not emissions greater than 10 MeV were
present. Since a uniform methodology was adopted for deriving the paramete
rs, this atlas should be very useful for future statistical and correlative
studies of solar flares.