Measurements of the lifetimes of electron bubbles in large size selected He-4(N)- droplets

Citation
M. Farnik et al., Measurements of the lifetimes of electron bubbles in large size selected He-4(N)- droplets, J CHEM PHYS, 110(18), 1999, pp. 9195-9201
Citations number
37
Categorie Soggetti
Physical Chemistry/Chemical Physics
Journal title
JOURNAL OF CHEMICAL PHYSICS
ISSN journal
00219606 → ACNP
Volume
110
Issue
18
Year of publication
1999
Pages
9195 - 9201
Database
ISI
SICI code
0021-9606(19990508)110:18<9195:MOTLOE>2.0.ZU;2-I
Abstract
The lifetimes of electron bubbles in large size selected He-4(N)- droplets have been measured in a molecular beam experiment to lie between 2 . 10(-3) and 0.2 s in droplets with sizes between N approximate to 10(5) and 10(7) atoms, respectively. The dependence of the lifetimes on the electric fields used to size select the droplets, on the energies of the incident electron s, and on the infrared radiation emitted from the apparatus walls were inve stigated and taken into account. The experimental lifetimes are many orders of magnitude smaller than predicted by earlier theories but consistent wit h a recent theory published by the authors in Phys. Rev. Lett. 81, 3892 (19 98. (C) 1999 American Institute of Physics. [S0021-9606(99)01016-8].