The carrier concentration dependence of the spin pseudogap phenomenon
in LaBa2Cu3Oy has been studied by means of the NMR/NQR method. From th
e T dependence of 1/T1T of the planar Cu site; it has turned out that
the characteristic temperature for the spin pseudogap at the staggered
mode is a monotonic function of hole concentration in the lightly dop
ed region. However, a spin-gap-like behavior was observed even in the
optimally doped sample (y = 6.96), where the maximal superconducting t
ransition temperature (T-c) is realized as a function of hole doping.
This feature is quite different from that in YBa2Cu3Oy, where the spin
pseudogap is restricted to the lightly doped region and is not observ
ed in the optimally doped sample (y = 6.98). Together with 1/T-2G and
Knight shift data, the nature of the gap is discussed.