Jp. Connerade et al., ATOMS IN CROSSED FIELDS - A NEW EXPERIMENTAL APPROACH, Journal of physics. B, Atomic molecular and optical physics, 30(9), 1997, pp. 2047-2066
We describe a novel experiment on Rydberg atoms in crossed electric an
d magnetic fields, recently performed at Imperial College. The novelty
resides in a combination of a crossed-field geometry with a time-gate
d detection technique, by which separation of the circularly polarized
components is now achieved. The importance of achieving such a separa
tion and the new opportunities it opens up an explained. By this appro
ach, a map of the diamagnetic Stark patterns is obtained. The data exh
ibit interesting behaviour in that the hydrogenic and non-hydrogenic g
roups within the n-shell now become distinguishable. Their evolution a
s a function of field strength brings out the difference between linea
r and quadratic effects. The levels with a quadratic dependence on ele
ctric held strength eventually invade and dominate the spectrum. We su
rmise that the trend from order to chaos is different in crossed field
s from the trend in the diamagnetic limit. We comment on further theor
y required to clarify this point. Our observations extend up to and sl
ightly above the saddle-point energy.