U. Mets et al., APPLICATION OF THE ANTIBUNCHING IN DYE FLUORESCENCE - MEASURING THE EXCITATION RATES IN SOLUTION, Chemical physics, 218(1-2), 1997, pp. 191-198
Experiments on antibunching in fluorescence of Rhodamine 6G in aqueous
solution have been carried out under optimized conditions. The depend
ence of the antibunching correlation times on the excitation intensity
has been studied, taking into account the saturation effects in the G
aussian intensity profile of the exciting laser beam. Information on t
he decay and excitation rates can be obtained and, with the knowledge
of the excitation intensity, the absorption cross-section can be estim
ated.