We study model electrorheological (ER) fluids which consist of three materi
al components in an attempt to explain recent experimental results, in whic
h the ER effects can be promoted by adding some water. At low water concent
ration, the droplets tend to aggregate on the surfaces of the dispersed par
ticles, forming coated microspheres. The ER effects are analyzed via spectr
al representation, and the experimental conditions for optimal ER responses
are obtained. At low frequencies, it is found that by tuning the thickness
and dielectric properties of the coating materials, it is possible to enha
nce the effective dielectric constant, thereby increasing the applicability
of the ER fluids.