Growing spatial correlations of particle displacements in a simulated liquid on cooling toward the glass transition

Citation
C. Donati et al., Growing spatial correlations of particle displacements in a simulated liquid on cooling toward the glass transition, PHYS REV L, 82(25), 1999, pp. 5064-5067
Citations number
26
Categorie Soggetti
Physics
Journal title
PHYSICAL REVIEW LETTERS
ISSN journal
00319007 → ACNP
Volume
82
Issue
25
Year of publication
1999
Pages
5064 - 5067
Database
ISI
SICI code
0031-9007(19990621)82:25<5064:GSCOPD>2.0.ZU;2-F
Abstract
We define a correlation function that quantifies the spatial correlation of single-particle displacements in liquids and amorphous materials. We show that for an equilibrium liquid this function is related to fluctuations in a bulk dynamical variable. We evaluate this function using computer simulat ions of an equilibrium glass-forming liquid, and show that long range spati al correlations of displacements emerge and grow on cooling toward the mode coupling critical temperature.