Fluid dynamics in microchannel reactors

Citation
S. Walter et al., Fluid dynamics in microchannel reactors, CHEM-ING-T, 71(5), 1999, pp. 447-455
Citations number
36
Categorie Soggetti
Chemical Engineering
Journal title
CHEMIE INGENIEUR TECHNIK
ISSN journal
0009286X → ACNP
Volume
71
Issue
5
Year of publication
1999
Pages
447 - 455
Database
ISI
SICI code
0009-286X(199905)71:5<447:FDIMR>2.0.ZU;2-Z
Abstract
The possible benefits of using microchannel reactors in the chemical proces s industries have been under discussion for several years. Outstanding heat transfer properties, short residence times and short diffusion lengths are considered key advantages, while the cost of the approach and the pending question of long-term stability are still major sources of skepticism. A go od starting point for a feasibility study is to investigate some major flui d dynamic properties. For a unit consisting of hundreds of parallel microch annels, the pressure drop for the laminar flow is just a few millibar. Howe ver, at high gas flows the distribution over the numerous channels may beco me non uniform. It is shown how the resulting residence time distribution a ffects both the yield of intermediates in consecutive reactions, and step f unctions of the concentration during periodic operation, respectively. All in all, the results of the estimations are encouraging.