X. Zhan et Jw. Brill, Frequency dependent shear compliance of TaS3: Depinning relaxation spectraand search for a glass transition, SYNTH METAL, 103(1-3), 1999, pp. 2671-2674
At T approximate to 100 K, the magnitude of the shear compliance of TaS3 in
creases by 25% with charge-density-wave (CDW) depinning by a de voltage. We
have measured the strain frequency dependence of the complex compliance (j
) at different voltages, and fit it to distributions of Debye relaxation mo
des. The sensitivity of the compliance to the structure of the CDW suggests
that it would also be sensitive to a glass transition. However, we find th
at both the real and imaginary parts of j are independent of frequency (wit
hin 1%) when the CDW remains pinned for 8 K < T < 70 K. j is also independe
nt (0.1%) of the frequency of small applied voltages, for which the dielect
ric constant varies greatly. Therefore, if there is a glass transition at t
hese temperatures, these results imply that either it does not involve rear
rangement of the CDW domain structure or that the elastic response time rem
ains > 1 s for the pinned CDW.