Frequency dependent shear compliance of TaS3: Depinning relaxation spectraand search for a glass transition

Authors
Citation
X. Zhan et Jw. Brill, Frequency dependent shear compliance of TaS3: Depinning relaxation spectraand search for a glass transition, SYNTH METAL, 103(1-3), 1999, pp. 2671-2674
Citations number
18
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science
Journal title
SYNTHETIC METALS
ISSN journal
03796779 → ACNP
Volume
103
Issue
1-3
Year of publication
1999
Pages
2671 - 2674
Database
ISI
SICI code
0379-6779(199906)103:1-3<2671:FDSCOT>2.0.ZU;2-2
Abstract
At T approximate to 100 K, the magnitude of the shear compliance of TaS3 in creases by 25% with charge-density-wave (CDW) depinning by a de voltage. We have measured the strain frequency dependence of the complex compliance (j ) at different voltages, and fit it to distributions of Debye relaxation mo des. The sensitivity of the compliance to the structure of the CDW suggests that it would also be sensitive to a glass transition. However, we find th at both the real and imaginary parts of j are independent of frequency (wit hin 1%) when the CDW remains pinned for 8 K < T < 70 K. j is also independe nt (0.1%) of the frequency of small applied voltages, for which the dielect ric constant varies greatly. Therefore, if there is a glass transition at t hese temperatures, these results imply that either it does not involve rear rangement of the CDW domain structure or that the elastic response time rem ains > 1 s for the pinned CDW.