R. Dorsinville et al., Nonlinear optical anisotropy in poly[3-(6-tetrahydropyraniloxyhexyl)]-2,5-thienylene Langmuir Blodgett films, SYNTH METAL, 101(1-3), 1999, pp. 204-205
The nonlinear optical response of Langmuir-Blodgett (LB) films of poly[3-(6
-tetrahydropyraniloxyhexyl)]-2, thienylene are investigated using degenerat
e four wave mixing techniques. A large third order nonlinear coefficient, c
hi((3)) similar to 10(-8) esu with subpicosecond response was observed. The
large value of chi((3)) is attributed to the longer conjugation length and
larger packing density of the LB films.