Diffusive convection driven by the differential diffusion of density alteri
ng fluid properties may enhance the scavenging of particles from natural bu
oyant plumes. For single-phase (fluid-solute-heat) systems this phenomenon
has been extensively studied because salt fingering generated at the oceani
c thermocline is a major mechanism of salt transport in the oceans. However
, the influence of this process on particle laden plumes, for example, fluv
ial plumes in lakes and estuaries volcanic clouds and seafloor hydrothermal
plumes is largely unknown. In this paper, we present direct experimental m
easurements of the interfacial particle flux at the plume base which can be
applied to predict particle scavenging from natural buoyant plumes, Partic
le flux is measured using a light attenuation technique employing a chain o
f photodiodes which average concentration over a large number of fingers. T
he results are in good general agreement with earlier studies based on fing
er velocity. Flux measurements cover a wide range of conditions from those
where diffusive convection dominates to those where settling and diffusive
convection are of a similar magnitude. For very small particles double diff
usive (salt finger) theory is applicable to two component particulate syste
ms as suggested by earlier studies [Green, T., 1987. The importance of doub
le diffusion to the settling of suspended material. Sedimentology 34, 319-3
31]. Two component diffusive convection theory is extended to three compone
nts in order to predict particle scavenging from marine fluvial plumes whic
h involve the diffusion of sediment, salt and heat. For larger particles wh
ich settle significantly the flux can be approximated by adding the double-
diffusive and settling fluxes. A theory to predict particle transport throu
gh the lower layer and sedimentation at the bed Is developed based on the o
bservation of strong convection below the plume. Application of our theory
and experimental results indicates that while double diffusion may signific
antly influence the longitudinal distribution and vertical sorting of depos
its from lacustrine plumes, the diffusive convection process is generally i
nsignificant in marine plumes. Observational evidence for lacustrine double
diffusion based on water column measurements is presented. (C) 1999 Elsevi
er Science B.V. All rights reserved.