P. Phanawadee et al., A new correlation for determination of the effective Knudsen diffusivity of a gas in a TAP reactor, IND ENG RES, 38(7), 1999, pp. 2877-2878
The analytical solution for the mean residence time of a nonreacting gas in
a three-zone TAP reactor packed with nonporous pellets is presented. It is
shown that the mean residence time is a sum of products of the weighting c
oefficient and reciprocal of the gas diffusivity of each zone. The weightin
g coefficients depend on the geometrical characteristics, i.e., lengths and
fractional voidages of the three zones. This simple equation is useful for
determination of the unknown gas diffusivity in the second zone (catalyst
zone) from an experimental diffusion response when diffusivities in the ine
rt-material zones (zone 1 and 3) are known.