The level structure of Th-227 has been studied using the alpha decay o
f U-231. The use of mass-separated U-231 sources and high-resolution a
lpha-particle and gamma-ray spectroscopy enabled the identification of
16 excited levels of (227)Tn. The angular distribution of alpha parti
cles in the decay of low-temperature oriented Th-227 is consistent wit
h a (227)Tn ground-state spin of 1/2. The low-lying levels of Th-227,a
n be interpreted in terms of a K = 1/2(+/-) parity doublet and a K = 3
/2(+) band coupled with the 1/2(+) member of the parity doublet by the
Coriolis interaction.