Two-colour phase control of gas harmonic generation has been demonstrated u
sing a 200-fs Ti:sapphire laser and its second harmonic. In the detection r
ange covering the 7th to the 20th harmonic order, a modulation of up to 27%
in the harmonic emission signal was observed by precisely varying the rela
tive phase between the two colours. Simulations based on the single-particl
e response predict enhancement of the high harmonic efficiency by orders of
magnitude for a given relative phase between the two colours.