Tk. Berntsen et al., Influence of Asian emissions on the composition of air reaching the North Western United States, GEOPHYS R L, 26(14), 1999, pp. 2171-2174
A global 3-D CTM has been used to study the impact of current and future em
issions from Asia on CO, PAN and O-3 across the North Pacific. Recent measu
rements from Washington State have been used to verify the model results wi
th respect to average concentrations as well as amplitude of perturbations
during episodic events of strong Asian influence. By performing CTM experim
ents with and without anthropogenic emissions from Asia, we find that there
is a significant contribution from Asian sources in the air arriving to th
e North Western United States, especially during spring. The mean contribut
ion, which can not easily be inferred from the available measurements, duri
ng spring are 34 ppbv, 26 pptv and 4 ppbv for CO, PAN and O-3 respectively.
The maximum enhancements caused by Asian sources during episodes are 42 pp
bv, 75 pptv, and 7.5 ppbv, respectively The amplitude of the perturbations
during short term (2-5 days) episodes of strong Asian influence are quite s
imilar to springtime Asian pollution events which have recently been observ
ed on the west coast of Washington state. A doubling of the current Asian e
missions in the model yields significant enhancements in all species, thoug
h not necessarily in a linear manner.