We present here the microwave surface impedance of a high-purity crystal of
YBa2Cu3O6.99 measured at five frequencies between 1 and 75 GHz. This data
set reveals the main features of the conductivity spectrum of the thermally
excited quasiparticles in the superconducting state. Below 20 K there is a
regime of extremely long quasiparticle scattering times, due to both the c
ollapse of inelastic scattering below T-c and the very weak impurity scatte
ring in the high-purity BaZrO3-grown crystal used in this study. Above 20 K
, the scattering increases dramatically, initially at least as fast as T-4.
[S0163-1829(99)04425-2].