Sr2Cu3O4Cl2 has Cu-I and Cu-II subsystems, forming interpenetrating S=1/2 s
quare lattice Heisenberg antiferromagnets. The classical ground state is de
generate, due to frustration of the intersubsystem interactions. Magnetic n
eutron scattering experiments show that quantum fluctuations cause a two di
mensional Ising ordering of the Cu-II's, lifting the degeneracy, and a dram
atic increase of the Cu-I out-of-plane spin-wave gap, unique for order out
of disorder. The spin-wave energies are quantitatively predicted by calcula
tions which include quantum fluctuations.