Neutron diffraction experiments were carried out to determine the magnetic
structure of Nd7Ni3 in an external field. At 4.2 K and in external fields b
elow 1.3 T the magnetic structure is conical with a basal plane helical com
ponent having a propagation vector Q = (0, 0, 1/3) and a c-axis ferromagnet
ic component. Above 1.3 T the c-axis component disappears, while the basal
plane component remains up to 2.7 T. Below 0.3 T, the magnetic structure ch
anges from conical to helical at about 8 K. A rough (H, T) phase diagram is
given and is generally consistent with the results of magnetization measur
ements. (C) 1999 Elsevier Science Ltd. All rights reserved.