Temperature-dependent magnetization measurements on a series of synthetic f
erritin proteins containing from 100 to 3000 Fe(III) ions are used to deter
mine the uncompensated moment of these antiferromagnetic particles. The res
ults are compared with recent theories of macroscopic quantum coherence whi
ch explicitly include the effect of this excess moment. The scaling of the
excess moment with protein size is consistent with a simple model of finite
-size effects and sublattice noncompensation. [S0163-1829(99)03429-3].