A new method for unfolding mean lifetimes and amplitudes as well as lifetim
e distributions from positron lifetime spectra is suggested and partially t
ested in this paper. The method is based on the use of artificial neural ne
tworks (ANNs). By using data from simulated positron spectra, generated by
a simulation program, an ANN can be trained to extract lifetimes and amplit
udes as well as their distributions from a positron spectrum as an input. I
n principle, the method has the potential to unfold an unknown number of li
fetimes and their distribution from a measured spectrum. So far, only a pro
of-of-principle type preliminary investigation was made by unfolding three
or four discrete Lifetimes. These investigations show that the task of desi
gning a proper and efficient network is not trivial. To achieve unfolding a
number of distributions requires both careful design of the network as wel
l as long training times. In addition, the performance of the method in pra
ctical applications is depending on the quality of the simulation model. Ho
wever, the chances of satisfying the above criteria appear to be good. When
appropriately developed, a trained network could be a very effective and e
fficient alternative to the existing methods, with very short identificatio
n times. (C) 1999 Elsevier Science B.V. All rights reserved.