magnetic properties of single-crystalline Tb2Fe17-xSix (x = 0, 1, 2, 3, and
3.3) have been investigated. The Si substitution constricted the lattices
by 1.5% and caused the Th2Ni17 transfer to Th2Zn17. The Curie temperature i
ncreased from 413 to 526 K, and the spontaneous magnetic moment decreased f
rom 82.6 to 46.4 emu/g with the increase of Si. The stronger anisotropy and
coercivity were generated by Si occupying the Fe sublattices. A domain wal
l pinning-dominated mechanism was responsible for increasing the coercivity
force from 0.01 T (x = 1) to about 0.36 T (x = 3.3) at 1.5 K.