Ii. Smolyaninov et al., Giant enhancement of surface second harmonic generation in BaTiO3 due to photorefractive surface wave excitation, PHYS REV L, 83(12), 1999, pp. 2429-2432
We report observation of strongly enhanced surface second harmonic generati
on (SHG) in BaTiO3 due to excitation of a photorefractive surface electroma
gnetic wave. Surface SH intensity may reach 10(-2) of the incident fundamen
tal light intensity. Angular, crystal orientation, and polarization depende
ncies of this SHG are presented. Possible applications of this effect in no
nlinear surface spectroscopy are discussed.