Ig. Koprinkov et al., High-energy conversion efficiency of transient stimulated Raman scatteringin methane pumped by the fundamental of a femtosecond Ti : sapphire laser, OPTICS LETT, 24(18), 1999, pp. 1308-1310
We studied stimulated Raman scattering in pressurized methane in the highly
transient regime pumped by 140-fs 0.7-mJ pulses from a Ti:sapphire (Ti:S)
laser tuned at 750 nm. Energy-conversion efficiency of the first Stokes of
more than 15% was achieved, with no strong sign of saturation with as much
as 40 atm (1 atm = 760 Torr) of Raman gas pressure. To our knowledge, this
is the highest conversion efficiency of transient stimulated Raman scatteri
ng generated directly from the fundamental of a Ti:S laser. (C) 1999 Optica
l Society of America. OCIS codes: 190.7110, 190.2640, 320.2250, 290.5910.