We find that harmonic generation can be enhanced with aperiodic optical sup
erlattice (AOS) structures realized by inverting poled ferroelectric domain
s in sample. The optimal design of the AOS can be achieved with use of the
simulated annealing method. The constructed AOSs can implement multiple wav
elength second-harmonic generation and the coupled third-harmonic generatio
n with an identical effective nonlinear coefficient. The simulations show t
hat the constructed AOSs can enhance harmonic generation compared with the
Fibonacci optical superlattice. The physical origin of this enhancement is
ascribed to the constructive interference effect. (C) 1999 American Institu
te of Physics. [S0003-6951(99)03841-3].