V. Kutzer et al., INTENSITY-DEPENDENT HOT-PHONON RELAXATION IN ZNSE, Materials science & engineering. B, Solid-state materials for advanced technology, 43(1-3), 1997, pp. 46-48
We performed time-resolved anti-Stokes Raman-scattering experiments on
ZnSe crystals using pump and probe techniques. To create non-equilibr
ium phonons we excited the ZnSe crystals at lambda = 632.8 nm with an
intense pump pulse with a pulse duration of about 4 ps, which leads to
efficient two-photon absorption and therefore to the creation of free
carriers. By relaxation to the band edge, the highly excited free car
riers emit longitudinal optical (LO) phonons, By varying the time dela
y between the probe and the pump pulse, the dynamical behavior of the
pump pulse-induced anti-Stokes Raman signal was studied. The results a
re discussed with respect to plasma effects influencing the dynamical
behavior of the phonon lifetime in ZnSe. (C) 1997 Elsevier Science S.A
.