Ft. Ferguson et Ja. Nuth, The influence of buoyant convection on the operation of the upward thermaldiffusion cloud nucleation chamber, J CHEM PHYS, 111(17), 1999, pp. 8013-8021
Recently, the stable operation of the upward thermal diffusion cloud chambe
r with respect to buoyancy-induced convection has become a concern in obtai
ning reliable nucleation data. During chamber operation, evidence of strong
convective currents are clearly visible due to the curved trajectories of
entrained droplets. A potential problem exists when these flows are much sm
aller in magnitude; there is no visible evidence of convection, yet these m
inute flows may result in systematic errors in the nucleation data calculat
ed via 1D diffusive models of the transport mechanisms within the chamber.
To examine whether such flows are possible and the characteristics of these
flows we have developed an extension to recent 2D modeling of the nucleati
on chamber which includes buoyancy-induced, convective motion. We have exam
ined both wet and dry chamber operation with an example case of 1-propanol
in helium at a pressure of 1.18 bar. In addition, for the dry wall case we
examined the effect of overheating the chamber wall and varying the chamber
diameter. Results indicate that, for the representative cases investigated
, very subtle convective flows can exist and that these minute flows can af
fect the maximum attainable supersaturation along the chamber centerline. F
inally, a list of general recommendations are given for minimizing the poss
ibility of such flows within the cloud chamber. (C) 1999 American Institute
of Physics. [S0021-9606(99)51833-3].