The influence of buoyant convection on the operation of the upward thermaldiffusion cloud nucleation chamber

Citation
Ft. Ferguson et Ja. Nuth, The influence of buoyant convection on the operation of the upward thermaldiffusion cloud nucleation chamber, J CHEM PHYS, 111(17), 1999, pp. 8013-8021
Citations number
19
Categorie Soggetti
Physical Chemistry/Chemical Physics
Journal title
JOURNAL OF CHEMICAL PHYSICS
ISSN journal
00219606 → ACNP
Volume
111
Issue
17
Year of publication
1999
Pages
8013 - 8021
Database
ISI
SICI code
0021-9606(19991101)111:17<8013:TIOBCO>2.0.ZU;2-C
Abstract
Recently, the stable operation of the upward thermal diffusion cloud chambe r with respect to buoyancy-induced convection has become a concern in obtai ning reliable nucleation data. During chamber operation, evidence of strong convective currents are clearly visible due to the curved trajectories of entrained droplets. A potential problem exists when these flows are much sm aller in magnitude; there is no visible evidence of convection, yet these m inute flows may result in systematic errors in the nucleation data calculat ed via 1D diffusive models of the transport mechanisms within the chamber. To examine whether such flows are possible and the characteristics of these flows we have developed an extension to recent 2D modeling of the nucleati on chamber which includes buoyancy-induced, convective motion. We have exam ined both wet and dry chamber operation with an example case of 1-propanol in helium at a pressure of 1.18 bar. In addition, for the dry wall case we examined the effect of overheating the chamber wall and varying the chamber diameter. Results indicate that, for the representative cases investigated , very subtle convective flows can exist and that these minute flows can af fect the maximum attainable supersaturation along the chamber centerline. F inally, a list of general recommendations are given for minimizing the poss ibility of such flows within the cloud chamber. (C) 1999 American Institute of Physics. [S0021-9606(99)51833-3].