Analytical solutions for the time-dependent autocorrelation function of the
classical and quantum mechanical spin dimer with arbitrary spin are presen
ted and compared. For large spin quantum numbers or high temperature the cl
assical and the quantum dimer become more and more similar, yet with the ma
jor difference that the quantum autocorrelation function is periodic in tim
e whereas the classical is not. (C) 1999 Elsevier Science B.V. All rights r
eserved.