We demonstrate femtosecond coherent control of excitons in quantum wel
ls with phase-locked pairs of 100 fs infrared pulses. Copolarized pump
pulses allow coherent control of exciton density and coherent destruc
tion of excitons within a few hundred femtoseconds of their creation.
This technique thus promises to avoid speed penalties in devices assoc
iated with long-lived persistent carrier populations, Cross-polarized
pump pulses allow coherent control of spin dynamics and conversion of
unpolarized excitons into spin polarized ones. Carrier density and spi
n are determined, respectively, from the differential reflection and f
rom the Faraday rotation of a third probe pulse. The experimental resu
lts are in good agreement with calculations based on the semiconductor
Bloch equations.