Two-color up-conversion time-resolved photoluminescence and time-resolved a
bsorption are used to study spin relaxation of near-resonant heavy-hole exc
itons in spontaneously ordered GaxIn1-xP. The photoluminescence anisotropy
is studied as a function of crystal direction, revealing a strong dependenc
e on the right orientation with respect to the ordering axis. The maximum o
bserved polarization is 0.8, and indicates that the polarization is near un
ity shortly after excitation. The carrier spin-relaxation time is 150 ps. [
S0163-1829(99)50940-5].