Using a microcalorimeter, we have measured the specific heat of C-60 and K3
C60 thin films from 6-400 K. The results can be understood by analyzing the
phonon modes; the electronic specific heat of K3C60 is a small fraction of
the total. While C-60 displays a clear separation of energy levels between
interball and intraball modes, the added (alkali) optical modes in K3C60 b
lur this separation because they appear in the gap. Additionally, the acous
tic modes of K3C60 soften compared to pure C-60. [S0163-1829(99)01039-5].