Electron spin resonance of defects in the Haldane system Y2BaNiO5

Citation
Cd. Batista et al., Electron spin resonance of defects in the Haldane system Y2BaNiO5, PHYS REV B, 60(18), 1999, pp. R12553-R12556
Citations number
15
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science
Journal title
PHYSICAL REVIEW B-CONDENSED MATTER
ISSN journal
01631829 → ACNP
Volume
60
Issue
18
Year of publication
1999
Pages
R12553 - R12556
Database
ISI
SICI code
0163-1829(19991101)60:18<R12553:ESRODI>2.0.ZU;2-B
Abstract
We calculate the electron paramagnetic resonance (EPR) spectra of the antif erromagnetic spin-1 chain compound Y2BaNi1-xMgxO5 for different values oft and temperature T much lower than the Haldane gap (similar to 100 K). The l ow-energy spectrum of an anisotropic Heisenberg Hamiltonian, with all param eters determined from experiment, has been solved using the density-matrix renormalization-group method. The observed EPR spectra are quantitatively r eproduced by this model. The presence of end-chain S = 1/2 states is clearl y observed as the main peak in the spectrum and the remaining structure is completely understood. [S0163-1829(99)50742-X].