Control of THz emission from Stark wave packets

Citation
Jl. Krause et Kj. Schafer, Control of THz emission from Stark wave packets, J PHYS CH A, 103(49), 1999, pp. 10118-10125
Citations number
35
Categorie Soggetti
Physical Chemistry/Chemical Physics
Journal title
JOURNAL OF PHYSICAL CHEMISTRY A
ISSN journal
10895639 → ACNP
Volume
103
Issue
49
Year of publication
1999
Pages
10118 - 10125
Database
ISI
SICI code
1089-5639(199912)103:49<10118:COTEFS>2.0.ZU;2-O
Abstract
We present calculations of the quantum control of THz emission from Stark w ave packets in sodium. Our method is based on the direct integration of the one-electron, time-dependent Schrodinger equation on a non-uniform, finite difference grid. We find that simple, experimentally feasible laser pulses are sufficient to optimize the frequency and intensity of the emitted THz radiation. A genetic algorithm is used to optimize the parameters of the ex citation pulse. Our results indicate that the dynamics, and hence the emitt ed radiation, depend sensitively on these parameters, and that the control space is rich and quite complicated.