C-induced Ge quantum dots grown by solid source molecular beam epitaxy was
investigated as functions of pre-deposited C coverage, overgrown Ge layer,
and substrate temperature using atomic force microscopy. It is observed tha
t the quantum dots grows with increasing pre-deposited C contents and they
also exhibit a bimodal size distribution. The smallest quantum dots with a
300 Angstrom mean diameter, a 50 Angstrom mean height, and an areal density
of 3.0x10(10) cm(-2) are obtained with 0.1 monolayer C pre-deposition and
a 3 monolayer thick Ge layer. We observed that an abrupt change in dot dens
ity and size occur near 500 degrees C, which is attributed to the differenc
e in the temperature-dependent surface diffusivities of Ge and C adatoms on
Si(100). These results suggest that C would be useful in obtaining achieve
much smaller quantum dots than Ge and SiGe dots on Si prepared using Stran
ski-Krastanov growth mode.