The thermal conductivity of ThO2 and Th0.98U0.02O2 was measured from 300-12
00 K. Calculations using a simple theoretical model show that the decrease
in thermal conductivity of Th0.98U0.02O2 over that of ThO2 is due to the en
hanced phonon-lattice strain interaction in the oxide. It is shown that the
intrinsic thermal resistivity arising due to phonon-phonon interaction in
these oxides can be quantitatively explained in terms of the modified Leibf
ried-Schlomann equation of Slack. (C) 2000 Elsevier Science B.V. All rights
reserved.