The ordered c(2 x 2) phase of Sn atoms on the Ni(100) surface was studied b
y constant-energy-loss electron-energy-loss holography (CEL-EELH). Three-di
mensional images at an atomic level around adsorbed Sn atoms of the surface
were deduced. The results clearly favour a chemisorption geometry with Sn
atoms incorporated into the first Ni layer, and demonstrate the ability of
the CEL-EELH technique to give atomic images similar to those obtained by s
ynchrotron radiation holography. (C) 2000 Published by Elsevier Science B.V
. All rights reserved.