Low-temperature thermodynamical properties of Bechgaard salts: (TMTSF)(2)PF6 versus (TMTSF)(2)AsF6

Citation
K. Biljakovic et al., Low-temperature thermodynamical properties of Bechgaard salts: (TMTSF)(2)PF6 versus (TMTSF)(2)AsF6, J PHYS IV, 9(P10), 1999, pp. 27-31
Citations number
16
Categorie Soggetti
Physics
Journal title
JOURNAL DE PHYSIQUE IV
ISSN journal
11554339 → ACNP
Volume
9
Issue
P10
Year of publication
1999
Pages
27 - 31
Database
ISI
SICI code
1155-4339(199912)9:P10<27:LTPOBS>2.0.ZU;2-Z
Abstract
We report on specific heat measurements of (TMTSF)(2)AsF6 in the temperatur e range 75 mK to 7 K and compare them with the results obtained for (TMTSF) (2)PF6. In addition to the generic features of density waves (DW) heat capa cities, there are similar discontinuities in the lattice contribution in bo th systems at 1.9 K and 3.5 K, which we ascribe to transitions between sub- SDW phases. The low-energy excitations (ZEE) contribution dominant at T<0.5 K, is strongly reduced in the case of AsF6 as well as the time dependent ef fects in the specific hear. We discuss the origin of the hyperfine T-2 term and give the arguments that it can only be provided by the metastable LEEs . Finally, we relate similarities but also differences, of the specific pro perties of mixed CDW/SDW states which has been recently found in structural investigations of both compounds.