K. Biljakovic et al., Low-temperature thermodynamical properties of Bechgaard salts: (TMTSF)(2)PF6 versus (TMTSF)(2)AsF6, J PHYS IV, 9(P10), 1999, pp. 27-31
We report on specific heat measurements of (TMTSF)(2)AsF6 in the temperatur
e range 75 mK to 7 K and compare them with the results obtained for (TMTSF)
(2)PF6. In addition to the generic features of density waves (DW) heat capa
cities, there are similar discontinuities in the lattice contribution in bo
th systems at 1.9 K and 3.5 K, which we ascribe to transitions between sub-
SDW phases. The low-energy excitations (ZEE) contribution dominant at T<0.5
K, is strongly reduced in the case of AsF6 as well as the time dependent ef
fects in the specific hear. We discuss the origin of the hyperfine T-2 term
and give the arguments that it can only be provided by the metastable LEEs
. Finally, we relate similarities but also differences, of the specific pro
perties of mixed CDW/SDW states which has been recently found in structural
investigations of both compounds.