A high-spatial-resolution dynamic experimental imaging setup, which can pro
vide simultaneous measurements of laser-induced frequency-domain infrared p
hotothermal radiometric and luminescence signals from defects in teeth, has
been developed for the first time. The major findings of this work are (i)
radiometric images are complementary to (anticorrelated with) luminescence
images, as a result of the nature of the two physical signal generation pr
ocesses; (ii) the radiometric amplitude exhibits much superior dynamic (sig
nal resolution) range to luminescence in distinguishing between intact and
cracked sub-surface structures in the enamel; (iii) the radiometric signal
(amplitude and phase) produces dental images with much better defect locali
zation, delineation, and resolution; (iv) radiometric images (amplitude and
phase) at a fixed modulation frequency are depth profilometric, whereas lu
minescence images are not; and (v) luminescence frequency responses from en
amel and hydroxyapatite exhibit two relaxation lifetimes, the longer of whi
ch (similar to ms) is common to all and is not sensitive to the defect stat
e and overall quality of the enamel. Simultaneous radiometric and luminesce
nce frequency scans for the purpose of depth profiling were performed and a
quantitative theoretical two-lifetime rate model of dental luminescence wa
s advanced. (C) 2000 Society of Photo-Optical Instrumentation Engineers. [S
1083-3668(00)00691-8].