The development of compact spectroscopic gas sensors and their applications
to environmental sensing will be described. These sensors employ mid-infra
red difference-frequency generation (DFG) in periodically poled lithium nio
bate (PPLN) crystals pumped by two single-frequency solid state lasers such
as diode lasers, diode-pumped solid state, and fiber lasers. Ultrasensitiv
e, highly selective, and real-time measurements of several important atmosp
heric trace gases, including carbon monoxide, nitrous oxide, carbon dioxide
, formaldehye, and methane, have been demonstrated.