A downer-riser circulating high velocity fluidization apparatus was develop
ed to study the fundamentals of downflowing gas-solid particle mixtures. Th
e acceleration and deceleration of solids due to the influences of the entr
ance and exit sections result in a relatively, uniform axial solids distrib
ution. Radial solid density profiles detected with an X-ray imaging system
in the downer show the existence of a core-annulus flow with a dilute cole
surrounded by a denser wall region. Local solids flux profiles were obtaine
d with an aspirating probe device and the solid velocity profile obtained f
rom the two measured ed quantities. These confirm that the majority of soli
ds segregates in a wall region that flows faster than the dilute core regio
n. Thus, the shorter residence time in the high-speed downer wall region is
coupled with faster reaction rates due to the accompanying high concentrat
ion of catalyst, while the dilute core has slower reaction rates with longe
r residence time due to the lower catalyst concentration and flow, velocity
. This results in much more uniform reaction extent over the cross-sectiona
l area of the downer and, therefore, should improve the product selectivity
.