Comparison of the lifetime of excited electrons in noble metals

Citation
R. Keyling et al., Comparison of the lifetime of excited electrons in noble metals, PHYS REV B, 61(3), 2000, pp. 1670-1673
Citations number
26
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science
Journal title
PHYSICAL REVIEW B
ISSN journal
10980121 → ACNP
Volume
61
Issue
3
Year of publication
2000
Pages
1670 - 1673
Database
ISI
SICI code
1098-0121(20000115)61:3<1670:COTLOE>2.0.ZU;2-8
Abstract
We present results for the lifetimes of hot electrons in the noble metals C u, Ag, and Au obtained by ab initio calculations within the framework of th e GW approximation. Our results show an overall good agreement with the ava ilable experimental data, especially for Ag. I,Cu and Au the experimental l ifetimes reveal, a sudden increase at low frequencies which cannot be expla ined within the GW approximation. For frequencies larger than 2 eV the calc ulated lifetimes are in good agreement with experiment. We also perform a d etailed comparison of our calculation with so-called "mass-shell" calculati ons.