A continuum model for non-dense growth

Citation
J. Los et al., A continuum model for non-dense growth, J PHYS-COND, 12(13), 2000, pp. 3195-3217
Citations number
27
Categorie Soggetti
Apllied Physucs/Condensed Matter/Materiales Science
Journal title
JOURNAL OF PHYSICS-CONDENSED MATTER
ISSN journal
09538984 → ACNP
Volume
12
Issue
13
Year of publication
2000
Pages
3195 - 3217
Database
ISI
SICI code
0953-8984(20000403)12:13<3195:ACMFNG>2.0.ZU;2-U
Abstract
We present a continuum model for diffusion-limited non-dense growth. Our ap proach leads to a set of two coupled partial differential equations which d escribe the time evolution of the (spherically) averaged aggregation densit y and concentration of growth units in the liquid phase. For time-independe nt parameters the solution of the equations yields a constant (non-fractal) aggregation density. The model gives a phenomenological description of non -fractal unstable growth, e.g. non-fractal spherulitic growth on a macrosco pic scale in terms of a minimal number of parameters and can be used in com bination with experimental data, such as the front velocity and the width o f the growth front, for both a qualitative and quantitative interpretation of the growth process. The analytical solution of the equations in the diff usion-limited regime leads to simple relations involving the aggregation de nsity and the velocity and width of the growth front. This allows for an ea sy quantitative analysis of experimental data.